13.-14.02.2020 Group seminar in Bacharach
13.12.2019: New paper available in ACP: Bozem et al. (2019)
Characterization of transport regimes and the polar dome during Arctic spring and summer using in situ aircraft measurements
The paper presents empirical trace gas based evidence on the location of the polar dome in the Canadian high Arctic. For this purpose airborne measurements of CO and CO2 during the NETCARE campaigns were analyzed to identify the transport barrier of the polar dome. It could be shown, that gradients of these species in isentropic and vertical direction mark the transport barrier of the polar dome. This clearly separates isolated innerarctic air masses from mid-latitude air. The distribution of 10-day backward trajectories confirms the existence of different air mass regimes as identified from the chemical composition. The trajectories further allow to identify characteristic transport processes for the air masses encountered during the different meteorological regimes. Based on the correlation between trace species an intermediate mixed regime could be identified during the summer campaign indicating exchange between the high arctic and mid latitudes.
10.12.2019: New paper available in Tellus B: Zanatta et al. (2019)
A new study led by Marco Zanatta (AWI) on trace gas and aerosol measurements over the Southern Baltic Sea is available in Tellus B. Our group contributed with airborne trace gas (CO2, O3) measurements and FLEXPART simulations.
28.11.2019: End of HALO SouthTRAC campaign
11.11.2019: HALO SouthTRAC campaign article in DFG magazine
29.10.2019: Special issue in ACP/AMT/WCD about isentropic exchange
More information: The Wave-driven ISentropic Exchange (WISE) mission is a collaborative research project to investigate transport and mixing processes in the upper troposphere and the lower stratosphere (UTLS) over the Atlantic. Headed by Forschungszentrum Jülich GmbH and the Johannes Gutenberg University of Mainz, 14 measurement flights were conducted with the high-altitude research aircraft HALO in September and October 2017 from Shannon, Ireland. Further partners providing instrumentation were the Karlsruhe Institute for Technology (KIT), the German Aerospace Center (DLR), the universities of Heidelberg, Frankfurt am Main, and Wuppertal, and the German National Metrology Institute. The scientific flights were supported by a team of about 90 persons.
The main objective of this project is to study the relation between chemical composition and the dynamical structure of the UTLS with a focus on the following topics: (i) interrelation of the tropopause inversion layer (TIL) and trace gas distribution, (ii) role of planetary wave breaking for water vapor transport into the extratropical lower stratosphere, (iii) role of halogenated substances for ozone and radiative forcing in the UTLS region, and (iv) occurrence and effects of sub-visual cirrus (SVC) in the lowermost stratosphere.
The special issue mainly includes papers from the airborne measurement campaign itself but is also open to other studies close to the topic. This includes both advanced scientific analyses of observational and measured data during the campaign as well as related climatological studies, but also manuscripts based on instrumental developments.
09.10.2019: New paper available in ACP: Kunkel et al. (2019)
Evidence of small-scale quasi-isentropic mixing in ridges of extratropical baroclinic waves
Stratosphere–troposphere exchange within extratropical cyclones provides the potential for anthropogenic and natural surface emissions to rapidly reach the stratosphere as well as for ozone from the stratosphere to penetrate deep into the troposphere, even down into the boundary layer. The efficiency of this process directly influences the surface climate, the chemistry in the stratosphere, the chemical composition of the extratropical transition layer, and surface pollution levels. Here, we present evidence for a mixing process within extratropical cyclones which has gained only a small amount of attention so far and which fosters the transport of tropospheric air masses into the stratosphere in ridges of baroclinic waves. We analyzed airborne measurement data from a research flight of the WISE (Wave-driven ISentropic Exchange) campaign over the North Atlantic in autumn 2017, supported by forecasts from a numerical weather prediction model and trajectory calculations. Further detailed process understanding is obtained from experiments of idealized baroclinic life cycles. The major outcome of this analysis is that air masses mix in the region of the tropopause and potentially enter the stratosphere in ridges of baroclinic waves at the anticyclonic side of the jet without changing their potential temperature drastically. This quasi-isentropic exchange occurs above the outflow of warm conveyor belts, in regions which exhibit enhanced static stability in the lower stratosphere and a Kelvin–Helmholtz instability across the tropopause. The enhanced static stability is related to radiative cooling below the tropopause and the presence of small-scale waves. The Kelvin–Helmholtz instability is related to vertical shear of the horizontal wind associated with small-scale waves at the upper edge of the jet stream. The instability leads to the occurrence of turbulence and consequent mixing of trace gases in the tropopause region. While the overall relevance of this process has yet to be assessed, it has the potential to significantly modify the chemical composition of the extratropical transition layer in the lowermost stratosphere in regions which have previously gained a small amount of attention in terms of mixing in baroclinic waves.
05.08.2019: Start of HALO SouthTRAC campaign
The project SouthTRAC (Southern Hemisphere Transport, Composition and Dynamics) will lead us together with several partners from FZ Jülich, KIT, DLR, University of Frankfurt, University of Wuppertal and University of Heidelberg and with funding from DFG to the southern tip of South America. Our destination and ground base in Argentina will be Rio Grande (53°47' S, 67°42' W).
We will have two intensive measurement periods in Rio Grande, one in September and the other in November. In between HALO will fly back to Oberpfaffenhofen/Germany. The goals of the mission are to study the composition of the UTLS over the Southern Hemisphere, gravity wave dynamics, as well as processes related to the Antarctic vortex.
More information on SouthTRAC can be found
20.5.2019: New paper available in ACP Kaluza et al. (2019)
Composite analysis of the tropopause inversion layer in extratropical baroclinic waves
The evolution of the tropopause inversion layer (TIL) during cyclogenesis in the North Atlantic storm track is investigated using operational meteorological analysis data (Integrated Forecast System from the European Centre for Medium-Range Weather Forecasts). For this a total of 130 cyclones have been analysed during the months August through October between 2010 and 2014 over the North Atlantic. Their paths of migration along with associated flow features in the upper troposphere and lower stratosphere (UTLS) have been tracked based on the mean sea level pressure field. Subsets of the 130 cyclones have been used for composite analysis using minimum sea level pressure to filter the cyclones based on their strength.
The composite structure of the TIL strength distribution in connection with the overall UTLS flow strongly resembles the structure of the individual cyclones. Key results are that a strong dipole in TIL strength forms in regions of cyclonic wrap-up of UTLS air masses of different origin and isentropic potential vorticity. These air masses are associated with the cyclonic rotation of the underlying cyclones. The maximum values of enhanced static stability above the tropopause occur north and northeast of the cyclone centre, vertically aligned with outflow regions of strong updraft and cloud formation up to the tropopause, which are situated in anticyclonic flow patterns in the upper troposphere. These regions are co-located with a maximum of vertical shear of the horizontal wind. The strong wind shear within the TIL results in a local minimum of Richardson numbers, representing the possibility for turbulent instability and potential mixing (or air mass exchange) within regions of enhanced static stability in the lowermost stratosphere.
15.4.2019: Kunkel et al. 2019: Paper on WISE mission at ACPD
One of the key topics of the WISE mission has been addressed by the Paper of D.Kunkel, who analyzes the occurrence of turbulence and mixing directly at the tropopause above the ridge region of an extratropical cyclone (https://www.atmos-chem-phys-discuss.net/acp-2019-342/). The paper bridges the in-situ observations with the fundamental process view from idealized simulations of baroclinic life cycles. These indicate that strong shear in regions of high static stability at the tropopause may lead to tracer exchange and mixing.
29.3.2019: Rhine-Main Universities undertake research on transport processes in the tropopause region
The Initiative Funding for Research of the Rhine-Main Universities (RMU) is currently supporting a cross-university project in the field of meteorology and climatology. The objective is to determine the time scales of transport processes in the tropopause, a region in the Earth's atmosphere at an elevation of 10 to 20 kilometers. The processes and composition in the tropopause region strongly affect surface temperatures and climate.
20. - 21. March 2019
The WISE group will meet for a data meeting from 20. - 21. March 2019 at Johannes Gutenberg University in Mainz.
22.2.2019: New Paper in ACP
A new study led by Hannes Schulz (AWI) on the vertical variability of black carbon (BC) in high Arctic spring and summer is available in ACP (https://www.atmos-chem-phys.net/19/2361/2019/). Our group contributed airborne carbon monoxide (CO) measurements and LAGRANTO kinematic back trajectories.
12.2.2019: Bozem et al. 2019 in ACPD
A new diagnostic for the determination of the polar dome boundary is presented using airborne in-situ CO and CO2 data as well as 10-day kinematic back trajectories in the European and Canadian Arctic in July 2014 and April 2015. Using the tracer derived boundary the analysis of the recent transport history of air masses within the polar dome reveals significant differences of dome extent and transport properties between spring and summer (https://www.atmos-chem-phys-discuss.net/acp-2019-70/).
19.11.2018: Kaluza et al., 2018 in ACPD
A new view on the static stability structure of extratropical cyclones is presented using a composite analysis of cyclones identified from ECMWF operational analysis data. The analysis shows, that even in regions of high static stability conditions favorable for cross tropopause exchange exist, which are linked to the occurrence of strong vertical shear of horizontal winds (https://www.atmos-chem-phys-discuss.net/acp-2018-1100/)
7 - 9 November 2018, OCTAV-UTLS workshop in Mainz
The 2nd meeting of the SPARC activity OCTAV-UTLS took place at the Helmholtz Institute (HIM) in Mainz. Speakers from the United States, UK, France and Gernany discussed new approaches and potential methods to account for the dynamical induced variability of ozone observations from different observations systems. These include radio sondes, LIDAR, aircraft measurements and satellite observations. The group defined a set of common diagnostic approaches to be applied to the different data sets, which allow to directly compare distributions and trends of ozone from different platforms and observational geometries consistently in the UTLS region. The comparison will be done at the next meeting in the United States at the Table Mountain lidar site.
13.10.2018: New discussion paper in ACPD
A summary paper about the advances of our understanding in the processes controlling Arctic aerosols during the NETCARE project led by Jonathan Abbatt (University of Toronto) and W. Richard Leaitch (Environment and Climate Change, Toronto) has been published for discussion in ACPD.
Our group contributed with airborne measurements during NETCARE 2014 and NETCARE 2015 as well as with FLEXPART simulations to analyze air mass histories.
02.10.2018: New discussion paper in ACPD
A new study led by Meng Si (University of British Columbia) on ice-nucleating particles in the Canadian High Arctic during spring 2016 is available in ACPD.
Our group provided FLEXPART results for a source attribution of the ice-nucleating particles.
01.-05.10.2018: SPARC General Assembly in Kyoto, Japan
31.08.2018: OCTAV-UTLS workshop, 7 - 9 November 2018, Mainz
The SPARC OCTAV - UTLS working group will meet for a data meeting from 7 - 9 November 2018 at the Johannes Gutenberg University in Mainz. We will host this meeting which will take place at the Helmholtz Institute Mainz (HIM).
More information can be found here.
24.08.2018: New discussion paper in ACPD
A new study led by Megan Willis (University of Toronto) on the vertical distribution of aerosols in the high Arctic is available now in ACPD.
Our group contributed airborne measurement data, ECMWF analysis data as well as results from FLEXPART simulations.
07.08.2018: HALO mission CAFE AFRICA started
Two member of our group, Franziska Köllner and Oliver Eppers, participate in the current HALO mission CAFE-AFRICA (lead: MPIC, Mainz) which is based on Cap Verde and studies the influence of the massive biomass burning emissions from southern Africa on the atmospheric oxidation capacity over the tropical and South Atlantic Ocean.
More information can be found here.